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A new strategy to identify the protein substrates of specific protein methyltransferases should allow scientists to better delineate the roles these signaling enzymes play in cells (J. Am. Chem. Soc., DOI: 10.1021/ja2118333). Methyltransferases, many of which are involved in gene transcription and epigenetic regulation, transfer a methyl group from an S-adenosyl-
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